Scalable manufacturing of fibrous nanocomposites for multifunctional liquid sensing

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dc.authorid0000-0002-5533-9621en_US
dc.authorid0000-0003-1570-0344en_US
dc.contributor.authorGoodman, Sheila M.
dc.contributor.authorTortajada, Ignacio Asensi
dc.contributor.authorHaslbeck, Florian
dc.contributor.authorOyulmaz, Kaan Yüksel
dc.contributor.authorDenizli, Haluk
dc.date.accessioned2023-06-26T19:42:20Z
dc.date.available2023-06-26T19:42:20Z
dc.date.issued2021en_US
dc.departmentBAİBÜ, Fen Edebiyat Fakültesi, Fizik Bölümüen_US
dc.descriptionThis research is supported by the Advanced Manufacturing Program (No. 1927623) from the National Science Foundation and by the McIntire-Stennis Cooperative Forestry Research Program (No. 1020630) from the USDA National Institute of Food and Agriculture. The authors also thank WestRock Paper Company for donated the wood pulp used in this research. Open access funding is enabled and organized by CERN.en_US
dc.description.abstractCellulose-based paper electronics is an attractive technology to meet the growing demands for naturally abundant, biocompatible, biodegradable, flexible, inexpensive, lightweight and highly miniaturizable sensory materials. The price reduction of industrial carbon nanotube (CNT) grades offers opportunities to manufacture electrically conductive papers whose resistivity is responsive to environmental stimuli, such as the presence of water or organic solvents. Here, a highly sensitive paper nanocomposite is developed by integrating CNTs into a hierarchical network of pulp fibers and nanofibrillated cellulose. The aqueous-phase dynamic web forming process enables the scalable production of sensory paper nanocomposites with minimal nanoparticle loss due to the tailored interfacial bonding between CNT and cellulose components. The resulting materials are applied as multifunctional liquid sensors, such as leak detection and wave monitoring. The sensitivity to liquid water spans an outstanding four orders of magnitude even after 30 cycles and 6-month natural aging, due to the hydroexpansion of the hierarchical cellulose network, which alters the intertube distance between neighboring CNTs. The re-organization of percolated CNTs modifies the electron transport in wet areas of the sheet, which can be predicted by an equivalent circuit of resistors for the rapid detection and quantification of various liquids over large surfaces. (c) 2021 Published by Elsevier Ltd.en_US
dc.description.sponsorshipNational Science Foundation [1927623]; USDA National Institute of Food and Agriculture [1020630]; CERN; Div Of Civil, Mechanical, & Manufact Inn; Directorate For Engineering [1927623] Funding Source: National Science Foundationen_US
dc.identifier.citationGoodman, S. M., Tortajada, I. A., Haslbeck, F., Oyulmaz, K. Y., Rummler, A., Sánchez, C. S., ... & Dichiara, A. B. (2021). Scalable manufacturing of fibrous nanocomposites for multifunctional liquid sensing. Nano Today, 40, 101270.en_US
dc.identifier.doi10.1016/j.nantod.2021.101270
dc.identifier.endpage8en_US
dc.identifier.issn1748-0132
dc.identifier.issn1878-044X
dc.identifier.scopus2-s2.0-85112841448en_US
dc.identifier.scopusqualityQ1en_US
dc.identifier.startpage1en_US
dc.identifier.urihttp://dx.doi.org/10.1016/j.nantod.2021.101270
dc.identifier.urihttps://hdl.handle.net/20.500.12491/11211
dc.identifier.volume40en_US
dc.identifier.wosWOS:000703392500001en_US
dc.identifier.wosqualityQ1en_US
dc.indekslendigikaynakWeb of Scienceen_US
dc.indekslendigikaynakScopusen_US
dc.institutionauthorOyulmaz, Kaan Yüksel
dc.institutionauthorDenizli, Haluk
dc.language.isoenen_US
dc.publisherElsevier Science Ltden_US
dc.relation.ispartofNano Todayen_US
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanıen_US
dc.rightsinfo:eu-repo/semantics/openAccessen_US
dc.subjectCellulose Nanofibrilsen_US
dc.subjectCarbon Nanotubesen_US
dc.subjectPaper-Based Electronicsen_US
dc.subjectLiquid Sensingen_US
dc.subjectLeak Detectionen_US
dc.titleScalable manufacturing of fibrous nanocomposites for multifunctional liquid sensingen_US
dc.typeArticleen_US

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