Investigation of hole-doping effect on structural, magnetic properties and magnetoresistance via Gd-site substitution by Pb in the layered manganite La0.1Gd0.2-xPbxCa1.2Sr0.6Mn2O7 (0 <= x <= 0.2)

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dc.authorid0000-0002-7280-6754en_US
dc.authorid0000-0002-3133-5693en_US
dc.authorid0000-0002-3133-5693en_US
dc.contributor.authorBelguet, Radjia
dc.contributor.authorMahamdioua, Nabil
dc.contributor.authorMeriche, Faiza
dc.contributor.authorAlonso, Jose A.
dc.contributor.authorMartinez, Jose L.
dc.contributor.authorAltıntaş, Sevgi Polat
dc.contributor.authorTerzioğlu, Cabir
dc.date.accessioned2024-03-07T13:11:22Z
dc.date.available2024-03-07T13:11:22Z
dc.date.issued2023en_US
dc.departmentBAİBÜ, Fen Edebiyat Fakültesi, Fizik Bölümüen_US
dc.descriptionThis work was supported by Directorate General for Scientific Research and Technological Development - Algeria,' and JAA and JLM thank the Spanish Ministry of Science and Innovation for granting the project numbers: PID2021-122477OB-I00, funded by MCIN/AEI/10.**13039/501100011033 and by ERDF A way of making Europe,' by the European Union.'en_US
dc.description.abstractIn this work, the hole-doping double-layered manganites with formula La1:0Gd(0.2-x)PbxCa1.2Sr0.6Mn2O7 (x = 0, 0.1, and 0.2) are prepared by the solidstate reaction route and experimentally characterized. The samples' crystallization into a tetragonal structure with an I4/mmm space group was confirmed by Rietveld refinement results of the XRD diffraction patterns using the FullProf software. The results were thoroughly studied after it was discovered that the cell parameters were decreasing. The structure was granular and porous, with grains that resembled spheres, according to micrographs obtained using a scanning electron microscope (SEM). Fourier-transform infrared (FTIR) analysis shows that our samples' characteristic vibrational bands are present. The entire temperature range of 0 to 300 K was used to evaluate electrical resistivity both in the absence and in the presence of an applied magnetic field. The increase in bandwidth, which is determined from the Rietveld refinement results, is found to explain why the rho(T) lowers with increasing Pb concentrations for a given temperature. The calculated magnetoresistance (MR%) for sample with x = 0.1 fell to 24.62% at 8 K for x = 0.2 from a maximum value of 30.01% at 5 K under 1 T of applied magnetic field. These values give our samples the opportunity to be good candidates in temperature and magnetic sensors in the cryogenic domains at low magnetic field. Residual resistivity, weak localization, electronelectron, and/or electron-phonon combinations fit the resistivity curves well in the low temperature region. The resistivity curves' fitting revealed that the adiabatic tiny polaron hopping model and Mott's 3D variable range hopping mechanism (3D-VRH) are both effective at controlling electrical conduction above T-MI and below Debye temperature, respectively. Based on Mott's 3D-VRH model, the density of states near the Fermi level (DOS), mean hopping distance Rh, and mean hopping energy E-h of the charge carriers have been carried out and discussed. On the basis of measurements of magnetization, inverse susceptibility, and loop hysteresis, the samples' magnetic properties are thoroughly described and discussed. The samples show a magnetic phase change from the ferromagnetic to the paramagnetic phase at Curie temperature T-C. Griffith phase temperature was determined to be above T-C based on the inverse of susceptibility's temperature dependency.en_US
dc.description.sponsorshipDirectorate General for Scientific Research and Technological Development - Algeria; Spanish Ministry of Science and Innovation - MCIN/AEI [PID2021-122477OB-I00]; ERDF A way of making Europe; European Unionen_US
dc.identifier.citationBelguet, R., Mahamdioua, N., Meriche, F., Alonso, J. A., Martinez, J. L., Denbri, F., ... & Terzioglu, C. (2023). Investigation of hole-doping effect on structural, magnetic properties and magnetoresistance via Gd-site substitution by Pb in the layered manganite La0. 1Gd0. 2− xPbxCa1. 2Sr0. 6Mn2O7 (0≤ x≤ 0.2). Journal of Materials Science: Materials in Electronics, 34(12), 1054.en_US
dc.identifier.doi10.1007/s10854-023-10452-4
dc.identifier.endpage24en_US
dc.identifier.issn0957-4522
dc.identifier.issn1573-482X
dc.identifier.issue12en_US
dc.identifier.scopus2-s2.0-85158074654en_US
dc.identifier.scopusqualityQ2en_US
dc.identifier.startpage1en_US
dc.identifier.urihttp://dx.doi.org/10.1007/s10854-023-10452-4
dc.identifier.urihttps://hdl.handle.net/20.500.12491/12061
dc.identifier.volume34en_US
dc.identifier.wosWOS:000985164300009en_US
dc.identifier.wosqualityQ2en_US
dc.indekslendigikaynakWeb of Scienceen_US
dc.indekslendigikaynakScopusen_US
dc.institutionauthorAltıntaş, Sevgi Polat
dc.institutionauthorTerzioğlu, Cabir
dc.language.isoenen_US
dc.publisherSpringeren_US
dc.relation.ispartofJournal of Materials Science: Materials in Electronicsen_US
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanıen_US
dc.rightsinfo:eu-repo/semantics/closedAccessen_US
dc.subjectRoom-Temperature Magnetoresistanceen_US
dc.subjectElectrical-Propertiesen_US
dc.subjectTransport-Propertiesen_US
dc.subjectMagnetocaloric Propertiesen_US
dc.subjectHopping Conductionen_US
dc.subjectCation Disorderen_US
dc.titleInvestigation of hole-doping effect on structural, magnetic properties and magnetoresistance via Gd-site substitution by Pb in the layered manganite La0.1Gd0.2-xPbxCa1.2Sr0.6Mn2O7 (0 <= x <= 0.2)en_US
dc.typeArticleen_US

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